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Journal Articles

Sorption behavior of niobium onto clay minerals in the presence of Ca

Ohira, Saki; Iida, Yoshihisa

Proceedings of Waste Management Symposia 2023 (WM2023) (Internet), 10 Pages, 2023/02

The sorption distribution coefficient (${it K}$d) of niobium-94 (Nb-94) on minerals is one of the important parameters in safety assessment of radioactive waste disposal. In a previous study, the ${it K}$d values of Nb under alkali condition in the presence of Ca, were two orders of magnitude higher than those in the presence of Na. In this study, Nb sorption experiments were performed to reexamine the effect of Ca on Nb sorption on clay minerals, and blank tests were performed to check for precipitation formation. The results showed that the Nb sorption onto montmorillonite and illite, did not depend on the Ca concentration, and ${it K}$d values obtained in the presence of Ca were the same as those in the absence of Ca. A sorption model assuming sorption by complexation on the mineral surface was developed and then calculated using the geochemical calculation code. The model with the surface species X_ONb(OH)$$_{4}$$ and X_ONb(OH)$$_{5}$$$$^{-}$$ represented trends in the data obtained.

Journal Articles

Laboratory experiment on runoff of particles deposited on land surface by rainfall at accidents in the decommissioning stage

Shimada, Taro; Namekawa, Masakazu*; Miwa, Kazuji; Takeda, Seiji

Proceedings of Waste Management Symposia 2023 (WM2023) (Internet), 8 Pages, 2023/02

It is supposed that radioactive dust deposited at the land surface will be moved downstream and concentrated at the depression by overland flow at heavy rain after the accidental release of radioactive dusts accumulated at the filters in the decommissioning stage of nuclear facilities. The authors are developing a calculation code to evaluate distribution changes of radioactivity on the surface and public dose considering the conditions such as rainfall, topography and types of cover surface. It is necessary to construct methods for setting parameter values used for the calculations based on the actual situation. Therefore, the parameter values were obtained by the experiments where Fe$$_3$$O$$_4$$ powder spread on the cover surface such as smooth and aged-asphalt, concrete and bare soil, was eroded by overland flow and raindrops and they were collected at the lower end of the slope at a minute interval. The collected weights of overland flow and Fe$$_3$$O$$_4$$ powder were measured. Based on the Manning's roughness coefficient for smooth asphalt already known as a fixed value, the erosion velocity coefficient was evaluated. Then Manning's roughness coefficients for other cover surfaces were obtained using the erosion velocity coefficient. Manning's roughness coefficients were slightly smaller than the range of literature values. In addition, elevations for the cover surface were measured by 3D scanner as point cloud data, and the surface roughness were evaluated. The values of surface roughness and Manning's roughness coefficients had a correlation. It indicated a possibility to utilize the surface roughness to set the Manning's roughness coefficient for the evaluation of radioactivity distribution change by heavy rainfall.

Journal Articles

LASSO reconstruction scheme to predict radioactive source distributions inside reactor building rooms; Theory & demonstration

Shi, W.*; Machida, Masahiko; Yamada, Susumu; Yoshida, Toru*; Hasegawa, Yukihiro*; Okamoto, Koji*

Proceedings of Waste Management Symposia 2023 (WM2023) (Internet), 8 Pages, 2023/02

Journal Articles

LASSO reconstruction scheme to predict radioactive source distributions inside reactor building rooms; Practical applications

Machida, Masahiko; Shi, W.*; Yamada, Susumu; Miyamura, Hiroko; Yoshida, Toru*; Hasegawa, Yukihiro*; Okamoto, Koji; Aoki, Yuto; Ito, Rintaro; Yamaguchi, Takashi; et al.

Proceedings of Waste Management Symposia 2023 (WM2023) (Internet), 11 Pages, 2023/02

Oral presentation

LASSO reconstruction scheme to predict radioactive source distributions inside reactor building rooms; Evaluation activities

Aoki, Yuto; Ito, Rintaro; Kitamura, Akihiro; Machida, Masahiko; Suzuki, Masahiro; Omori, Takazumi; Taniguchi, Tatsuro; Ide, Hiroshi

no journal, , 

Oral presentation

LASSO reconstruction scheme to predict radioactive source distributions inside reactor building rooms; Outline of R&D project

Suzuki, Masahiro; Aoki, Yuto; Machida, Masahiko; Ito, Rintaro; Kawabata, Kuniaki; Yamaguchi, Takashi; Okamoto, Koji

no journal, , 

Oral presentation

R&D project of digital techniques to reduce radiation exposure for Fukushima Daiichi decommissioning; Overview and key results

Suzuki, Masahiro; Machida, Masahiko; Ito, Rintaro; Kawabata, Kuniaki; Yamaguchi, Takashi; Okamoto, Koji

no journal, , 

no abstracts in English

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